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High-pressure Raman study of vibrational spectra in crystalline acetanilide
http://hdl.handle.net/2298/9616
http://hdl.handle.net/2298/9616753a4e57-4f74-4e43-83ff-c4302b929314
名前 / ファイル | ライセンス | アクション |
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PRB_047_0150.pdf (692.0 kB)
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Item type | 学術雑誌論文 / Journal Article(1) | |||||
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公開日 | 2008-10-23 | |||||
タイトル | ||||||
タイトル | High-pressure Raman study of vibrational spectra in crystalline acetanilide | |||||
言語 | ||||||
言語 | eng | |||||
キーワード | ||||||
主題 | crystalline acetanilide, 結晶アセトアニリド, vibrational spectra, 振動スペクトル, high-pressure Raman, 高圧ラマン, self-trapping, セルフトラッピング, diamond anvil cell, ダイヤモンドアンビルセル | |||||
資源タイプ | ||||||
資源タイプ | journal article | |||||
著者 |
酒井, 政道
× 酒井, 政道× Kuroda, Noritaka× 仁科, 雄一郎 |
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別言語の著者 |
酒井, 政道
× 酒井, 政道× 黒田, 規敬× 仁科, 雄一郎 |
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内容記述 | ||||||
内容記述 | We have studied the effect of pressure on the low-frequency lattice modes and the amide-I (N-C?O stretching) vibrational modes in crystalline acetanilide (C6H5NHCOCH3) in the temperature range 80–300 K by means of Raman spectroscopy. The Raman intensity of the 1650-cm-1 band, which appears upon cooling, is enhanced by applying pressure. The energy difference between the amide-I phonon (Ag mode) and the 1650-cm-1 bands does not change appreciably under pressure up to at least 4 GPa. These results are analyzed in terms of the self-trapped model in which a single lattice mode couples with the amide-I excitation by taking into account the effect of pressure on the low-frequency lattice modes and on the dipole-dipole interactions associated with the amide-I vibration. A band is observed at 30 cm-1 below the amide-I phonon band at low temperatures with a pressure above ∼2 GPa. | |||||
内容記述 | ||||||
内容記述 | 有機分子性結晶特有の分子振動と格子振動の結合形態をアセトアニリド結晶についてラマン散乱により実験的に調査した。実験は大気圧下と、ダイヤモンドアンビルセルを用いた加圧下で、室温から80 Kまでの範囲で精密に温度を変えて行った。その結果、アミド-I分子振動モードが格子振動と結合して自己束縛を起こした振舞いを明瞭に観測することができ、分子・格子結合のメカニズムを解明するとともに、結合定数を定量的に評価することができた。 | |||||
書誌情報 |
Physical Review B 巻 47, 号 1, p. 150-157, 発行年 1993-01-01 |
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ISSN | ||||||
収録物識別子 | 01631829 | |||||
書誌レコードID | ||||||
収録物識別子 | AA00362255 | |||||
DOI | ||||||
関連タイプ | isIdenticalTo | |||||
関連識別子 | 10.1103/PhysRevB.47.150 | |||||
権利 | ||||||
権利情報 | ©1993 The American Physical Society | |||||
フォーマット | ||||||
内容記述 | application/pdf | |||||
形態 | ||||||
691955 bytes | ||||||
著者版フラグ | ||||||
出版タイプ | VoR | |||||
日本十進分類法 | ||||||
主題 | 431.5 | |||||
その他の言語のタイトル | ||||||
その他のタイトル | アセトアニリド結晶における振動スペクトルの高圧ラマン研究 | |||||
タイトル(ヨミ) | ||||||
その他のタイトル | アセトアニリド ケッショウ ニ オケル シンドウ スペクトル ノ コウアツ ラマン ケンキュウ | |||||
出版者 | ||||||
出版者 | The American Physical Society | |||||
資源タイプ | ||||||
内容記述 | 論文(Article) | |||||
資源タイプ・ローカル | ||||||
雑誌掲載論文 | ||||||
資源タイプ・NII | ||||||
Journal Article | ||||||
資源タイプ・DCMI | ||||||
text | ||||||
資源タイプ・ローカル表示コード | ||||||
01 | ||||||
URL | ||||||
内容記述 | http://link.aps.org/abstract/PRB/v47/p150 | |||||
コメント | ||||||
黒田規敬: 熊本大学大学院自然科学研究科マテリアル工学講座・工学部マテリアル工学科 |